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cture like most salts at warmer temperatures between 140 and 150 c for cshso 4 some solid acids undergo a phase transition to become highly disordered superprotonic structures which increases conductivity by several orders of magnitude safc systems use cesium dihydrogen phosphate csh 2 po 4 and have demonstrated lifetimes in the thousands of hours 39 alkaline fuel cell edit main articles alkaline fuel cell and alkaline anion exchange membrane fuel cell the alkaline fuel cell afc or hydrogen oxygen fuel cell was designed and first demonstrated publicly by francis thomas bacon in 1959 it was used as a primary source of electrical energy in the apollo space program 40 the cell consists of two porous carbon electrodes impregnated with a suitable catalyst such as pt ag coo etc the space between the two electrodes is filled with a concentrated solution of koh or naoh which serves as an electrolyte h 2 gas and o 2 gas are bubbled into the electrolyte through the porous carbon electrodes thus the overall reaction involves the combination of hydrogen gas and oxygen gas to form water the cell runs continuously until the reactant s supply is exhausted this type of cell operates efficiently in the temperature range 343 413 k 70 140 c and provides a potential of about 0 9 v 41 alkaline anion exchange membrane fuel cell aaemfc is a type of afc which employs a solid polymer electrolyte instead of aqueous potassium hydroxide koh and it is superior to aqueous afc high temperature fuel cells edit solid oxide fuel cell edit main article solid oxide fuel cell solid oxide fuel cells sofcs use a solid material most commonly a ceramic material called yttria stabilized zirconia ysz as the electrolyte because sofcs are made entirely of solid materials they are not limited to the flat plane configuration of other types of fuel cells and are often designed as rolled tubes they require high operating temperatures 800 1000 c and can be run on a variety of fuels including natural gas 6 sofcs are unique because negatively charged oxygen ions travel from the cathode positive side of the fuel cell to the anode negative side of the fuel cell instead of protons travelling vice versa i e from the anode to the cathode as is the case in all other types of fuel cells oxygen gas is fed through the cathode where it absorbs electrons to create oxygen ions the oxygen ions then travel through the electrolyte to react with hydrogen gas at the anode the reaction at the anode produces electricity and water as by products carbon dioxide may also be a by product depending on the fuel but the carbon emissions from a sofc system are less than those from a fossil fuel combustion plant 42 the chemical reactions for the sofc system can be expressed as follows 43 anode reaction 2h 2 2o 2 2h 2 o 4e cathode reaction o 2 4e 2o 2 overall cell reaction 2h 2 o 2 2h 2 o sofc systems can run on fuels other than pure hydrogen gas however since hydrogen is necessary for the reactions listed above the fuel selected must contain hydrogen atoms for the fuel cell to operate the fuel must be converted into pure hydrogen gas sofcs are capable of internally reforming light hydrocarbons such as methane natural gas 44 propane and butane 45 these fuel cells are at an early stage of development 46 challenges exist in sofc systems due to their high operating temperatures one such challenge is the potential for carbon dust to build up on the anode which slows down the internal reforming process research to address this carbon coking issue at the university of pennsylvania has shown that the use of copper based cermet heat resistant materials made of ceramic and metal can reduce coking and the loss of performance 47 another disadvantage of sofc systems is the long start up making sofcs less useful for mobile applications despite these disadvantages a high operating temperature provides an advantage by removing the need for a precious metal catalyst like platinum thereby reducing cost additionally waste heat from sofc systems may be captured and reused increasing the theoretical overall efficiency to as high as 80 85 6 the high operating temperature is largely due to the physical properties of the ysz electrolyte as temperature decreases so does the ionic conductivity of ysz therefore to obtain the optimum performance of the fuel cell a high operating temperature is required according to their website ceres power a uk sofc fuel cell manufacturer has developed a method of reducing the operating temperature of their sofc system to 500 600 degrees celsius they replaced the commonly used ysz electrolyte with a cgo cerium gadolinium oxide electrolyte the lower operating temperature allows them to use stainless steel instead of ceramic as the cell substrate which reduces cost and start up time of the system 48 molten carbonate fuel cell edit main article molten carbonate fuel cell molten carbonate fuel cells mcfcs require a high operating temperature 650 c 1 200 f similar to sofcs mcfcs use lithium potassium carbonate salt as an electrolyte and this salt liquefies at high temperatures allowing for the movement of charge within the cell in this case negative carbonate ions 49 like sofcs mcfcs are capable of converting fossil fuel to a hydrogen rich gas in the anode eliminating the need to produce hydrogen externally the reforming process creates co 2 emissions mcfc compatible fuels include natural gas biogas and gas produced from coal the hydrogen in the gas reacts with carbonate ions from the electrolyte to produce water carbon dioxide electrons and small amounts of other chemicals the electrons travel through an external circuit creating electricity and return to the cathode there oxygen from the air and carbon dioxide recycled from the anode react with the electrons to form carbonate ions that replenish the electrolyte completing the circuit 49 the chemical reactions for an mcfc system can be expressed as follows 50 anode reaction co 3 2 h 2 h 2 o co 2 2e cathode reaction co 2 ½o 2 2e co 3 2 overall cell reaction h 2 ½o 2 h 2 o as with sofcs mcfc disadvantages include slow start up times because of their high operating temperature this makes mcfc systems not suitable for mobile applications and this technology will most likely be used for stationary fuel cell purposes the main challenge of mcfc technology is the cells short life span the high temperature and carbonate electrolyte lead to corrosion of the anode and cathode these factors accelerate the degradation of mcfc components decreasing the durability and cell life researchers are addressing this problem by exploring corrosion resistant materials for components as well as fuel cell designs that may increase cell life without decreasing performance 6 mcfcs hold several advantages over other fuel cell technologies including their resistance to impurities they are not prone to carbon coking which refers to carbon build up on the anode that results in reduced performance by slowing down the internal fuel reforming process therefore carbon rich fuels like gases made from coal are compatible with the system the united states department of energy claims that coal itself might even be a fuel option in the future assuming the system can be made resistant to impurities such as sulfur and particulates that result from converting coal into hydrogen 6 mcfcs also have relatively high efficiencies they can reach a fuel to electricity efficiency of 50 considerably higher than the 37 42 efficiency of a phosphoric acid fuel cell plant efficiencies can be as high as 65 when the fuel cell is paired with a turbine and 85 if heat is captured and used in a combined heat and power chp system 49 fuelcell energy a connecticut based fuel cell manufacturer develops and sells mcfc fuel cells the company says that their mcfc products range from 300 kw to 2 8 mw systems that achieve 47 electrical efficiency and can utilize chp technology to obtain higher overall efficiencies one product the dfc erg is combined with a gas turbine and according to the company it achieves an electrical efficiency of 65 51 electric storage fuel cell edit the electric storage fuel cell is a conventional battery chargeable by electric power input using the conventional electro chemical effect however the battery further includes hydrogen and oxygen inputs for alternatively charging the battery chemically 52 biofuel cell edit main articles microbial fuel cell and enzymatic biofuel cell a biofuel cell converts chemical energy from biological substances into electrical energy using biological catalysts such as enzymes or microorganisms the process involves the oxidation of a fuel like glucose at the anode releasing electrons and protons the electrons travel through an external circuit to generate electrical current while at the cathode oxygen is typically reduced to water or hydrogen peroxide completing the circuit 53 applications include wastewater treatment and renewable energy production 54 conductive polymers may be used to improve electron transfer between enzymes and electrodes 55 the integration of nanomaterials such as carbon nanotubes and metal nanoparticles are used to enhance the performance of bfcs these materials increase the surface area of electrodes and facilitate better electron transfer resulting in higher power densities three dimensional porous structures and graphene based materials have been used to improve conductivity and stability and hybrid biofuel cells that combine bfcs with supercapacitors or secondary batteries are being developed to provide stable and continuous energy output 56 bfcs are being explored as power sources for implantable devices like pacemakers and biosensors to potentially eliminate the need for traditional batteries and fiber type ebfcs show potential in implantable applications 57 the power density of bfcs however is generally lower than that of conventional energy sources the stability of enzymes and microorganisms over extended periods is another concern and scalability and commercial viability also pose hurdles 58 comparison of fuel cell types edit fuel cell name electrolyte qualified power w working temperature c efficiency status cost usd w cell system electro galvanic fuel cell aqueous alkaline solution 40 commercial research 3 7 direct formic acid fuel cell dfafc polymer membrane ionomer 50 w 40 commercial research 10 20 alkaline fuel cell aqueous alkaline solution 10 200 kw 80 60 70 62 commercial research 50 100 proton exchange membrane fuel cell polymer membrane ionomer 1 w 500 kw 50 100 nafion 59 120 200 pbi 60 50 70 30 50 61 commercial research 50 100 metal hydride fuel cell aqueous alkaline solution 20 50 p peak 0 c commercial research 30 200 zinc air battery aqueous alkaline solution 40 mass production 150 300 direct carbon fuel cell several different 700 850 80 70 commercial research 18 direct borohydride fuel cell aqueous alkaline solution 70 commercial 400 450 microbial fuel cell polymer membrane or humic acid 40 research 10 50 upflow microbial fuel cell umfc 40 research 1 5 regenerative fuel cell polymer membrane ionomer 50 commercial research 200 300 direct methanol fuel cell polymer membrane ionomer 100 mw 1 kw 90 120 20 30 10 25 61 commercial research 125 reformed methanol fuel cell polymer membrane ionomer 5 w 100 kw 250 300 reformer 125 200 pbi 50 60 25 40 commercial research 8 50 direct ethanol fuel cell polymer membrane ionomer 140 mw cm² 25 90 120 research 12 redox fuel cell broken anchor rfc liquid electrolytes with redox shuttle and polymer membrane ionomer 1 kw 10 mw research 12 50 phosphoric acid fuel cell molten phosphoric acid h 3 po 4 10 mw 150 200 55 40 61 co gen 90 commercial research 4 00 4 50 solid acid fuel cell h conducting oxyanion salt solid acid 10 w 1 kw 200 300 55 60 40 45 commercial research 15 molten carbonate fuel cell molten alkaline carbonate 100 mw 600 650 55 45 55 61 commercial research 1000 tubular solid oxide fuel cell tsofc o 2 conducting ceramic oxide 100 mw 850 1100 60 65 55 60 commercial research 3 50 protonic ceramic fuel cell h conducting ceramic oxide 700 research 80 planar solid oxide fuel cell o 2 conducting ceramic oxide 100 mw 500 1100 60 65 55 60 61 commercial research 800 enzymatic biofuel cells any that will not denature the enzyme 40 research 10 magnesium air fuel cell salt water 20 to 55 90 commercial research 15 glossary of terms in table further information glossary of fuel cell terms anode the electrode at which oxidation a loss of electrons takes place for fuel cells and other galvanic cells the anode is the negative terminal for electrolytic cells where electrolysis occurs the anode is the positive terminal 62 aqueous solution 63 of relating to or resembling water made from with or by water catalyst a chemical substance that increases the rate of a reaction without being consumed after the reaction it can potentially be recovered from the reaction mixture and is chemically unchanged the catalyst lowers the activation energy required allowing the reaction to proceed more quickly or at a lower temperature in a fuel cell the catalyst facilitates the reaction of oxygen and hydrogen it is usually made of platinum powder very thinly coated onto carbon paper or cloth the catalyst is rough and porous so the maximum surface area of the platinum can be exposed to the hydrogen or oxygen the platinum coated side of the catalyst faces the membrane in the fuel cell 62 cathode the electrode at which reduction a gain of electrons occurs for fuel cells and other galvanic cells the cathode is the positive terminal for electrolytic cells where electrolysis occurs the cathode is the negative terminal 62 electrolyte a substance that conducts charged ions from one electrode to the other in a fuel cell battery or electrolyzer 62 fuel cell stack individual fuel cells connected in a series fuel cells are stacked to increase voltage 62 matrix something within or from which something else originates develops or takes form 64 membrane the separating layer in a fuel cell that acts as electrolyte an ion exchanger as well as a barrier film separating the gases in the anode and cathode compartments of the fuel cell 62 molten carbonate fuel cell mcfc a type of fuel cell that contains a molten carbonate electrolyte carbonate ions co 3 2 are transported from the cathode to the anode operating temperatures are typically near 650 c 62 phosphoric acid fuel cell pafc a type of fuel cell in which the electrolyte consists of concentrated phosphoric acid h 3 po 4 protons h are transported from the anode to the cathode the operating temperature range is generally 160 220 c 62 proton exchange membrane fuel cell pem a fuel cell incorporating a solid polymer membrane used as its electrolyte protons h are transported from the anode to the cathode the operating temperature range is generally 60 100 c for low temperature proton exchange membrane fuel cell lt pemfc 62 pem fuel cell with operating temperature of 120 200 c is ...
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